Determination of the isotopic ratio 236U/238U in Austrian water samples

Autor(en)

Michaela Srncik, Peter Steier, Gabriele Wallner

Abstrakt

236U with a half life of 2.3 × 107 years is naturally produced in ultra-trace amounts (236U/238U <10-10) in ores, soils and rocks, while a huge amount has been produced in nuclear power plants and possibly nuclear weapons tests by man. Thus, anthropogenic uranium may cause a significant measurement background for geological applications of natural 236U. To investigate this background, water samples from rivers, creeks and wells were collected in the alpine region of Forstau (Salzburg, Austria) and from surrounding areas. Thin sources for alpha spectrometry were prepared by anion exchange and co-precipitation with NdF3 to determine the 238U concentration. These filters were reprocessed for the analysis of the isotopic ratio 236U/238U by AMS. The special aim was the characterization of the 236U/238U ratio in natural waters and the investigation of contributions from anthropogenic sources. Our measurements of 236U in Austrian water samples from wells, rivers and creeks show the first data on the spreading of anthropogenic 236U in the general environment far from local contamination sources.

Organisation(en)

Institut für Anorganische Chemie, Isotopenphysik

Journal

Nuclear Instruments & Methods in Physics Research. Section B. Beam Interactions with Materials and Atoms

Band

268

Seiten

1146-1149

Anzahl der Seiten

4

ISSN

0168-583X

DOI

https://doi.org/10.1016/j.nimb.2009.10.120

Publikationsdatum

2010

Peer-reviewed

Ja

ÖFOS 2012

104003 Anorganische Chemie, 104020 Radiochemie

Link zum Portal

https://ucris.univie.ac.at/portal/de/publications/determination-of-the-isotopic-ratio-236u238u-in-austrian-water-samples(d6b2b9de-1987-4a82-9d72-3890e8059946).html